Graphitization induced structural transformation of candle soot carbon into carbon nano-onion as a functional anode for metal-ion batteries

Pathak, Anil D. and Potphode, Darshna and Sharma, Chandra Shekhar (2022) Graphitization induced structural transformation of candle soot carbon into carbon nano-onion as a functional anode for metal-ion batteries. Materials Advances, 3 (8). pp. 3610-3619. ISSN 2633-5409

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Abstract

This work reports for the first time the structural transformation of glassy spherical candle soot carbon into graphitic polyhedral carbon nano-onions (multilayer fullerenes) by simple graphitization of candle soot carbon at varying temperatures from 1500 to 2400 °C. This structural transformation of candle soot carbon is thoroughly investigated by high-resolution transmission electron microscopy, X-ray diffraction, and Raman spectroscopy, with the aid of first-principles calculation based on density functional theory to understand the effect on physiochemical properties. Further, this understanding of structural transformation enables a promising pathway to tune the electrochemical properties of graphitized candle soot carbon to develop it as a functional anode for metal-ion (Li-ion as well K-ion) battery applications. © 2022 The Author(s).

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IITH Creators:
IITH CreatorsORCiD
Sharma, Chandra Shekharhttps://orcid.org/0000-0003-3821-1471
Item Type: Article
Uncontrolled Keywords: glassy spherical candle soot carbon, graphitic polyhedral carbon nano-onions (multilayer fullerenes), high-resolution transmission electron microscopy, X-ray diffraction, and Raman spectroscopy.
Subjects: Chemical Engineering
Divisions: Department of Chemical Engineering
Depositing User: . LibTrainee 2021
Date Deposited: 21 Jul 2022 08:40
Last Modified: 21 Jul 2022 08:40
URI: http://raiith.iith.ac.in/id/eprint/9839
Publisher URL: http://doi.org/10.1039/d2ma00042c
OA policy: https://v2.sherpa.ac.uk/id/publication/41211
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